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HomeMy WebLinkAboutDRC-2025-001670299 South Main Street, Suite 1700 Salt Lake City, Utah 84111 (801) 649-2000 Fax: (801) 880-2879 www.energysolutions.com May 19, 2025 CD-2025-107 Mr. Doug Hansen, Director Division of Waste Management and Radiation Control 195 North 1950 West Salt Lake City, UT 84114-4880 Subject: Federal Cell Facility Application: Responses to Round 2 Request for Information (per DRC- 2025-001480) Dear Mr. Hansen: EnergySolutions hereby responds to the Utah Division of Waste Management and Radiation Control’s May, 8 2025 (DRC-2025-001480) Requests for Information (RFI) on our Federal Cell Facility Application. A response is provided for each request using the Director’s assigned reference number. Each RFI letter is addressed individually, with the text of the RFI quoted in bold italics followed by its response. Multiple follow-up RFI letters are addressed in this response, with each letter preceded by a solid line. The following attachments are also electronically provided to this response submission. 1. FOLDER: Reference to AB-7b-1 Response 2. FOLDER: RESRAD Input and Output Appendix AB: Operational Period Modeling AB-7,b-1: (from DRC-2025-001480): The review of revision 3 of Appendix AB and NAC-0023_R7 confirmed that the RESRAD-OFFSITE inventory has been updated. Revision 3 of Appendix AB states, “Because DU PA v4.0 includes distributions for uranium isotopes from both SRS and GDP populations, the higher concentrations from GDP waste were used for U-234, U-235, U-236, and U-238. The GDP waste does not report U-233 concentrations, so SRS waste is used here.” After comparing the reported U- 234, U-235, U-236, and U-238 concentrations of SRS waste and GDP waste in NAC-0023_R7, it was confirmed that the GDP waste concentrations are higher for U-234, U-235, and U-238, but SRS waste has a higher U-236 concentration than GDP waste (GDP = 2.17E+2 pCi/g; SRS = 4.91E+3 pCi/g). In review of the spreadsheet “DU waste concs and RESRAD results-Feb 2025.xlsx,” it was found that in the calculations for the RESRAD-OFFSITE radionuclide inventory, the lower U-236 concentration for GDP waste was used with the SRS mass. For U-234, U-235, and U-238, the higher GDP concentrations were used with the GDP mass. Please rerun the model with the updated inventory to use the higher SRS U-236 concentration in these calculations. A screening calculation of potential radionuclide concentrations in the groundwater, surface water, biota, and air pathways is conducted for the Federal Cell Facility using the waste inventory and other applicable parameters from the Depleted Uranium (DU) PA v4.0. The Mr. Doug Hansen CD-2025-107 May 19, 2025 Page 2 of 12 modeling is performed using RESRAD-OFFSITE version 4.0. Parameter values are tabulated below. An operational period of 20 years is assumed1. The operational period model assumes that a groundwater well is located 90 ft from the edge of the contaminated zone, and applies DU PA model Kd values for silty sand (contaminated zone and vadose zone; Unit 3), silty clay (liner material and pond sediment; Unit 4), and clay (saturated zone; Unit 2) as well as DU model physical characteristics for the waste disposal layer and the vadose and saturated zones. The RESRAD-OFFSITE model requires that the volume of the contaminated zone be constant. The operational period analysis incorporates the simplifying assumption that the time-averaged concentrations of disposed radionuclides in the contaminated zone during the emplacement period are one-half of the waste concentrations. Practically, this has the effect of protectively overestimating potential releases in the first half of the operating period. The release of radionuclides from the disposed waste over time is protectively modeled as occurring immediately upon placement, such that functionally no “credit” is taken for the integrity of waste containers. In summary, the following protective assumptions are invoked: 1. the time-averaged disposed waste inventory for the Federal Cell is assumed to exist beginning at model year 0 (the beginning of disposal operations); and, 2. radionuclides are assumed to be freely available for environmental transport based on instantaneous equilibrium desorption from soil-like material, as defined by Kd values; Because there are no natural surface water bodies in the vicinity of the site, EnergySolutions’ permitted artificial evaporation pond constructed to store runoff water during active disposal operations is evaluated. A surface water evaporation pond with an area of 88,200 ft 2 (EnergySolutions 2000) and an average volume of 2.2 million gallons (EnergySolutions 2020 annual groundwater report values for the permitted 2000 Evaporation Pond (EnergySolutions 2021a)) is assumed to be the receiving medium for radionuclides transported with runoff from the Federal Cell during the operational period. Retained evaporation pond sediments will be disposed at the time of site closure. As noted above, all radionuclides are assumed to exist within a soil-like material and the surface erosion rate from the Federal Cell footprint to the evaporation pond is assumed to be 0.001 cm/yr, based on combined gully and sheet erosion modeling performed for the PA. Radionuclide concentrations in the open disposal cell were derived from the DU PA v4.02 GoldSim model. The initial inventory of each radionuclide in the disposal cell at the time of closure was assigned to the volume of the closed disposal cell (338,500 m 3) and was expressed as activity per unit mass using the dry bulk density of silty sand (Unit 3) and DU 1 RESRAD-Offsite was run for 50 years so results are available for longer operational periods, if desired. In this report, results are displayed to 25 years to facilitate evaluating trends, if any, beyond the assumed 20-year operational period. 2 Because DU PA v4.0 includes distributions for uranium isotopes from both SRS and GDP populations, the higher concentrations from GDP waste were used for U-234, U-235, and U-238. The GDP waste does not report U-233 concentrations, so SRS waste is used here. See tab “Inventory Conv.” in the Excel file “DU waste concs and RESERAD results-May2025.xlsx.” Mr. Doug Hansen CD-2025-107 May 19, 2025 Page 3 of 12 waste applied in the GoldSim model (1.609 g/cm 3). As described above, one-half of the as- disposed radionuclide concentrations were used in the RESRAD-OFFSITE modeling to represent average concentrations across the virtual 2.4-m thick zone of primary contamination. The derivation of the time-averaged radionuclide concentrations used in the RESRAD-OFFSITE modeling is shown in Table 1 below. Table 1 - Time-Averaged Radionuclide Concentrations Used in the RESRAD-OFFSITE Modeling Species Initial Inventory (Bq) Initial Concentration (Bq/g) Initial Concentration (pCi/g) Time-Averaged Concentration (pCi/g) Sr-90 3.77E+10 6.93E-02 1.87E+00 0.94 Tc-99 3.22E+13 5.91E+01 1.60E+03 799 I-129 1.49E+10 2.74E-02 7.41E-01 0.37 Cs-137 9.71E+09 1.78E-02 4.82E-01 0.24 Ra-226 6.09E+08 1.12E-03 3.02E-02 0.015 U-233 4.25E+12 7.80E+00 2.11E+02 105 U-234 9.98E+14 1.83E+03 4.95E+04 24772 U-235 9.06E+13 1.66E+02 4.50E+03 2249 U-236 3.94E+12 7.24E+00 1.96E+02 98 U-238 5.81E+15 1.07E+04 2.88E+05 144076 Np-237 4.56E+09 8.37E-03 2.26E-01 0.11 Pu-238 1.69E+08 3.10E-04 8.37E-03 0.0042 Pu-239 1.03E+09 1.89E-03 5.10E-02 0.025 Pu-240 2.73E+08 5.01E-04 1.35E-02 0.0068 Pu-241 3.24E+09 5.95E-03 1.61E-01 0.08 Am-241 1.14E+10 2.09E-02 5.66E-01 0.28 Modeling of transport to groundwater and a surface water retention pond was conducted for several open disposal cell geometries. The dimensions evaluated include: a) a 100 × 100 ft area (30.48 m × 30.48 m [929 m 2]); b) one-quarter of the disposal cell (133.5 m × 239.5 m [3.2E+04 m 2]); c) one-half of the disposal cell (267 m × 239.5 m [6.4E+04 m 2]); and d) the entire footprint of the DU waste disposal cell (267 m × 479 m [1.3E+05 m 2]). Model results were output at the following model years: 1, 5, 10, 15, 20, and 25 years. The assumed operational period is 20 years. Results are shown to 25 years to facilitate evaluating trends, if any, beyond year 20. Among the isotopes of uranium, results are shown for uranium-238. Because physical transport characteristics are identical for all the long-lived uranium isotopes, the other uranium isotopes would show identical characteristics with their Mr. Doug Hansen CD-2025-107 May 19, 2025 Page 4 of 12 modeled concentrations in various media proportional to their initial inventory. Based on initial inventory and transport characteristics, results are also shown for radium-226 (the parent of radon-222) and the highly soluble radionuclide technetium-99. 1. Well Water Radionuclide Concentrations. No breakthrough of any radionuclides at the well located 90 ft from the edge of the contaminated zone occurs within 25 years for any of the four open operational area cases evaluated. Even assuming no cover is placed on the disposed DU waste, and taking no credit for containerization, breakthrough of Tc-99 at the well does not occur until model year 200 in the RESRAD-OFFSITE evaluation. Other radionuclides do not see breakthrough within 500 years. Longer-term modeling of releases to groundwater from the closed disposal cell is the subject of the DU PA. Figure 1. No Breakthrough at 90-ft Well from Edge of Contaminated Zone. Mr. Doug Hansen CD-2025-107 May 19, 2025 Page 5 of 12 2. Radon Flux above Open DU Waste. Radon-222 flux above the open area of the disposal cell, based on decay of the Ra-226 parent, is independent of the assumed dimensions of the open portion of the disposal cell during operations. Modeled radon flux is based on the assumption that containers do not restrict release of radon gas, and the radium-226 source concentration in the DU waste is represented as a time-averaged concentration in a homogenous soil source of 2.4-m thickness. The initial ground surface flux of approximately 0.01216 pCi/m2-s decreases very slightly to about 0.01203 pCi/m2-s at model year 25. The rate at which radon-222 flux decreases is roughly proportional to the 1,600-year half-life of radium-226. Figure 2. Radon-222 Flux Above the Open Area of the Disposal Cell, Mr. Doug Hansen CD-2025-107 May 19, 2025 Page 6 of 12 3. Concentrations of Particulate-Phase Radionuclides in Air above Open DU Waste. Concentrations of radionuclides above the assumed soil source term of the open disposal cell are modeled using default RESRAD-OFFSITE particulate resuspension and atmospheric mixing assumptions. Air concentrations are directly proportional to the virtual soil concentrations of these radionuclides, and these concentrations are essentially static across the modeling period. Although not evident on the scale of the plots, the radium-226 air particulates concentration decreases slightly over time in the same manner as radon-222 flux. Figure 3. Particulate Air Concentrations above a 929 m2 (100 ft x 100 ft) Open Disposal Area Mr. Doug Hansen CD-2025-107 May 19, 2025 Page 7 of 12 Figure 4. Particulate Air Concentrations above a 3.2E+04 m2 (Quarter Cell) Open Disposal Area Figure 5. Particulate Air Concentrations above a 6.4E+04 m2 (Half Cell) Open Disposal Area Mr. Doug Hansen CD-2025-107 May 19, 2025 Page 8 of 12 Figure 6. Particulate Air Concentrations above a 1.3E+05 m2 (Full Cell) Open Disposal Area 4. Concentrations of Radionuclides in Retention Pond Water. Radionuclide transport to the retention pond through erosion of the open disposal area by runoff and atmospheric deposition is tracked through modeled water concentrations, which are in equilibrium with pond sediments having an assumed active partitioning layer of 10-cm thickness. Pond water concentrations of radionuclides increase quickly and then begin to level off over time as incoming sediments eventually comprise all of the 10-cm mixing layer on the pond bottom. Technetium-99 reaches 90% of its pond water value at model year 25 by approximately year 12, and radium-226 pond concentrations reach 90% of their model year 25 value by model year 17. For uranium isotopes, 90% of peak pond water concentrations occur at approximately model year 14. Concentrations of radionuclides in pond water are directly proportional to the assumed size of the open operational area. Figure 7. Radionuclide Concentrations in Retention Pond Water for a 929 m2 (100 ft x 100 ft) Open Disposal Area Mr. Doug Hansen CD-2025-107 May 19, 2025 Page 9 of 12 Figure 8. Radionuclide Concentrations in Retention Pond Water for a 3.2E+04 m2 (Quarter Cell) Open Disposal Area Figure 9. Radionuclide Concentrations in Retention Pond Water for a 6.4E+04 m2 (Half Cell) Open Disposal Area Mr. Doug Hansen CD-2025-107 May 19, 2025 Page 10 of 12 Figure 10. Radionuclide Concentrations in Retention Pond Water for a 1.3E+05 m2 (Full Cell) Open Disposal Area 5. 5. Concentrations of Radionuclides in Retention Pond Crustacea. RESRAD-OFFSITE includes modeling of radionuclide uptake into fish and crustacea inhabiting a surface water body. The stormwater retention body is assumed to host small invertebrates, which are represented by crustacea in the RESRAD-OFFSITE model. Crustacea tissue concentrations are modeled in RESRAD based on element-specific partitioning among three media: pond water, pond sediment, and crustacean tissue. Over the 25-year modeling period, modeled concentrations in pond crustacea (assuming any exist) follow a similar pattern to pond water. As with pond water, concentrations of radionuclides in the tissues of crustacea are directly proportional to the assumed size of the open operational area. Figure 11. Radionuclide Concentrations in Retention Pond Crustacea for a 929 m2 (100 ft x 100 ft) Open Disposal Area Mr. Doug Hansen CD-2025-107 May 19, 2025 Page 11 of 12 Figure 12. Radionuclide Concentrations in Retention Pond Crustacea for a 3.2E+04 m2 (Quarter Cell) Open Disposal Area Figure 13. Radionuclide Concentrations in Retention Pond Crustacea for a 6.4E+04 m2 (Half Cell) Open Disposal Area Mr. Doug Hansen CD-2025-107 May 19, 2025 Page 12 of 12 Figure 14. Radionuclide Concentrations in Retention Pond Crustacea for a 1.3E+05 m2 (Full Cell) Open Disposal Area If you have further questions regarding these responses to the director’s request of DRC-2025- 001480, please contact me at (801) 649-2000. Sincerely, Vern C. Rogers Director, Regulatory Affairs Electronic enclosures I certify under penalty of law that this document and all attachments were prepared under my direction or supervision in accordance with a system designed to assure that qualified personnel properly gather and evaluate the information submitted. Based on my inquiry of the person or persons who manage the system, or those persons directly responsible for gathering the information, the information submitted is, to the best of my knowledge and belief, true, accurate, and complete. I am aware that there are significant penalties for submitting false information, including the possibility of fine and imprisonment for knowing violations.